Water's structure on material surfaces, known as self-organized water (SOW), exhibits unique properties and charge separation, showing potential for scientific insights and practical applications. Recent studies indicate that electromagnetic energy, particularly infrared light, can influence and enlarge SOWs, suggesting a key role for energy in regulating interfacial water. The transition to renewable energy sources is vital, with hydrogen emerging as a promising option for energy storage and distribution. Hydrogen production through water electrolysis using renewable energy could significantly reduce emissions, driving increased research in scaling up this technology. Researchers are focusing on the role of SOW in enhancing hydrogen evolution reaction (HER) performance, showcasing improved efficiency and proton transport through SOW structures. The study highlights how SOW stabilization of transition states via dipole alignment impacts local electric fields, improving electrolysis efficiency. By customizing interfacial water structures, the research bridges biological water studies with electrochemical applications, offering insights into enhancing catalysis and optimizing proton-transfer processes. The study introduces a self-organized water electrolyzer with PEO-coated platinum electrodes, demonstrating enhanced efficiency, stability, and scalability for integration with renewable sources like solar and wind energy, paving the way for sustainable energy technology.